Cliff Robertson

Cole Younger

Robert Duvall

Jesse James

Luke Askew

Jim Younger

R. G. Armstrong

Clell Miller

Dana Elcar

Allen

Donald Moffat

Manning

John Pearce

Frank James

Matt Clark

Bob Younger

Wayne Sutherlin

Charley Pitts

Robert H. Harris

Wilcox

Jack Manning

Heywood

Elisha Cook Jr.

Bunker (as Elisha Cook)

Royal Dano

Gustavson

Mary-Robin Redd

Kate

William Callaway

Calliopist

Arthur Peterson

Jefferson Jones

Craig Curtis

Chadwell

Barry Brown

Henry Wheeler

Nellie Burt

Doll Woman

Liam Dunn

Drummer

Madeleine Taylor Holmes

Granny Woman

Herbert Nelson

Chief Detective

Erik Holland

Sheriff

Anne Barton

Clell's Wife

Marjorie Durant

Maybelle

Inger Stratton

Singing Whore

Valda Hansen

Nude Girl (as Valda J. Hansen)

Pamela Collins

Kate's Girl (uncredited)